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Precision instrument bolsters efforts to find elusive dark energy

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Precision instrument bolsters efforts to find elusive dark energy


Dark energy — a mysterious force pushing the universe apart at an ever-increasing rate — was discovered 26 years ago, and ever since, scientists have been searching for a new and exotic particle causing the expansion.

Pushing the boundaries of this search, University of California, Berkeley physicists have now built the most precise experiment yet to look for minor deviations from the accepted theory of gravity that could be evidence for such a particle, which theorists have dubbed a chameleon or symmetron.

The experiment, which combines an atom interferometer for precise gravity measurements with an optical lattice to hold the atoms in place, allowed the researchers to immobilize free-falling atoms for seconds instead of milliseconds to look for gravitational effects, besting the current most precise measurement by a factor of five.

Though the researchers found no deviation from what is predicted by the theory spelled out by Isaac Newton 400 years ago, expected improvements in the precision of the experiment could eventually turn up evidence that supports or disproves theories of a hypothetical fifth force mediated by chameleons or symmetrons.

The ability of the lattice atom interferometer to hold atoms for up to 70 seconds — and potentially 10 times longer — also opens up the possibility of probing gravity at the quantum level, said Holger Müller, UC Berkeley professor of physics. While physicists have well-tested theories describing the quantum nature of three of the four forces of nature — electromagnetism and the strong and weak forces — the quantum nature of gravity has never been demonstrated.

“Most theorists probably agree that gravity is quantum. But nobody has ever seen an experimental signature of that,” Müller said. “It’s very hard to even know whether gravity is quantum, but if we could hold our atoms 20 or 30 times longer than anyone else, because our sensitivity increases with the second or fourth power of the hold time, we could have a 400 to 800,000 times better chance of finding experimental proof that gravity is indeed quantum mechanical.”

Aside from precision measurements of gravity, other applications of the lattice atom interferometer include quantum sensing.

“Atom interferometry is particularly sensitive to gravity or inertial effects. You can build gyroscopes and accelerometers,” said UC Berkeley postdoctoral fellow Cristian Panda, who is first author of a paper about the gravity measurements set to be published this week in the journal Nature and is co-authored by Müller. “But this gives a new direction in atom interferometry, where quantum sensing of gravity, acceleration and rotation could be done with atoms held in optical lattices in a compact package that is resilient to environmental imperfections or noise.”

Because the optical lattice holds atoms rigidly in place, the lattice atom interferometer could even operate at sea, where sensitive gravity measurements are employed to map the geology of the ocean floor.

Screened forces can hide in plain sight

Dark energy was discovered in 1998 by two teams of scientists: a group of physicists based at Lawrence Berkeley National Laboratory, led by Saul Perlmutter, now a UC Berkeley professor of physics, and a group of astronomers that included UC Berkeley postdoctoral fellow Adam Riess. The two shared the 2011 Nobel Prize in Physics for the discovery.

The realization that the universe was expanding more rapidly than it should came from tracking distant supernovas and using them to measure cosmic distances. Despite much speculation by theorists about what’s actually pushing space apart, dark energy remains an enigma — a large enigma, since about 70% of the entire matter and energy of the universe is in the form of dark energy.

One theory is that dark energy is merely the vacuum energy of space. Another is that it is an energy field called quintessence, which varies over time and space.

Another proposal is that dark energy is a fifth force much weaker than gravity and mediated by a particle that exerts a repulsive force that varies with the density of surrounding matter. In the emptiness of space, it would exert a repulsive force over long distances, able to push space apart. In a laboratory on Earth, with matter all around to shield it, the particle would have an extremely small reach.

This particle has been dubbed a chameleon, as if it’s hiding in plain sight.

In 2015, Müller adapted an atom interferometer to search for evidence of chameleons using cesium atoms launched into a vacuum chamber, which mimics the emptiness of space. During the 10 to 20 milliseconds it took the atoms to rise and fall above a heavy aluminum sphere, he and his team detected no deviation from what would be expected from the normal gravitational attraction of the sphere and Earth.

The key to using free-falling atoms to test gravity is the ability to excite each atom into a quantum superposition of two states, each with a slightly different momentum that carries them different distances from a heavy tungsten weight hanging overhead. The higher momentum, higher elevation state experiences more gravitational attraction to the tungsten, changing its phase. When the atom’s wave function collapses, the phase difference between the two parts of the matter wave reveals the difference in gravitational attraction between them.

“Atom interferometry is the art and science of using the quantum properties of a particle, that is, the fact that it’s both a particle and a wave. We split the wave up so that the particle is taking two paths at the same time and then interfere them at the end,” Müller said. “The waves can either be in phase and add up, or the waves can be out of phase and cancel each other out. The trick is that whether they are in phase or out of phase depends very sensitively on some quantities that you might want to measure, such as acceleration, gravity, rotation or fundamental constants.”

In 2019, Müller and his colleagues added an optical lattice to keep the atoms close to the tungsten weight for a much longer time — an astounding 20 seconds — to increase the effect of gravity on the phase. The optical lattice employs two crossed laser beams that create a lattice-like array of stable places for atoms to congregate, levitating in the vacuum. But was 20 seconds the limit, he wondered?

During the height of the COVID-19 pandemic, Panda worked tirelessly to extend the hold time, systematically fixing a list of 40 possible roadblocks until establishing that the wiggling tilt of the laser beam, caused by vibrations, was a major limitation. By stabilizing the beam within a resonant chamber and tweaking the temperature to be a bit colder — in this case less than a millionth of a Kelvin above absolute zero, or a billion times colder than room temperature — he was able to extend the hold time to 70 seconds.

He and Müller published those results in the June 11, 2024, issue of Nature Physics.

Gravitational entanglement

In the newly reported gravity experiment, Panda and Müller traded a shorter time, 2 seconds, for a greater separation of the wave packets to several microns, or several thousandths of a millimeter. There are about 10,000 cesium atoms in the vacuum chamber for each experiment — too sparsely distributed to interact with one another — dispersed by the optical lattice into clouds of about 10 atoms each.

“Gravity is trying to push them down with a force a billion times stronger than their attraction to the tungsten mass, but you have the restoring force from the optical lattice that’s holding them, kind of like a shelf,” Panda said. “We then take each atom and split it into two wave packets, so now it’s in a superposition of two heights. And then we take each one of those two wave packets and load them in a separate lattice site, a separate shelf, so it looks like a cupboard. When we turn off the lattice, the wave packets recombine, and all the quantum information that was acquired during the hold can be read out.”

Panda plans to build his own lattice atom interferometer at the University of Arizona, where he was just appointed an assistant professor of physics. He hopes to use it to, among other things, more precisely measure the gravitational constant that links the force of gravity with mass.

Meanwhile, Müller and his team are building from scratch a new lattice atom interferometer with better vibration control and a lower temperature. The new device could produce results that are 100 times better than the current experiment, sensitive enough to detect the quantum properties of gravity. The planned experiment to detect gravitational entanglement, if successful, would be akin to the first demonstration of quantum entanglement of photons performed at UC Berkeley in 1972 by the late Stuart Freedman and former postdoctoral fellow John Clauser. Clauser shared the 2022 Nobel Prize in Physics for that work.

Other co-authors of the gravity paper are graduate student Matthew Tao and former undergraduate student Miguel Ceja of UC Berkeley, Justin Khoury of the University of Pennsylvania in Philadelphia and Guglielmo Tino of the University of Florence in Italy. The work is supported by the National Science Foundation (1708160, 2208029), Office of Naval Research (N00014-20-1-2656) and Jet Propulsion Laboratory (1659506, 1669913).



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Early dark energy could resolve cosmology’s two biggest puzzles

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Precision instrument bolsters efforts to find elusive dark energy


A new study by MIT physicists proposes that a mysterious force known as early dark energy could solve two of the biggest puzzles in cosmology and fill in some major gaps in our understanding of how the early universe evolved.

One puzzle in question is the “Hubble tension,” which refers to a mismatch in measurements of how fast the universe is expanding. The other involves observations of numerous early, bright galaxies that existed at a time when the early universe should have been much less populated.

Now, the MIT team has found that both puzzles could be resolved if the early universe had one extra, fleeting ingredient: early dark energy. Dark energy is an unknown form of energy that physicists suspect is driving the expansion of the universe today. Early dark energy is a similar, hypothetical phenomenon that may have made only a brief appearance, influencing the expansion of the universe in its first moments before disappearing entirely.

Some physicists have suspected that early dark energy could be the key to solving the Hubble tension, as the mysterious force could accelerate the early expansion of the universe by an amount that would resolve the measurement mismatch.

The MIT researchers have now found that early dark energy could also explain the baffling number of bright galaxies that astronomers have observed in the early universe. In their new study, reported in the Monthly Notices of the Royal Astronomical Society, the team modeled the formation of galaxies in the universe’s first few hundred million years. When they incorporated a dark energy component only in that earliest sliver of time, they found the number of galaxies that arose from the primordial environment bloomed to fit astronomers’ observations.

You have these two looming open-ended puzzles,” says study co-author Rohan Naidu, a postdoc in MIT’s Kavli Institute for Astrophysics and Space Research. “We find that in fact, early dark energy is a very elegant and sparse solution to two of the most pressing problems in cosmology.”

The study’s co-authors include lead author and Kavli postdoc Xuejian (Jacob) Shen, and MIT professor of physics Mark Vogelsberger, along with Michael Boylan-Kolchin at the University of Texas at Austin, and Sandro Tacchella at the University of Cambridge.

Big city lights

Based on standard cosmological and galaxy formation models, the universe should have taken its time spinning up the first galaxies. It would have taken billions of years for primordial gas to coalesce into galaxies as large and bright as the Milky Way.

But in 2023, NASA’s James Webb Space Telescope (JWST) made a startling observation. With an ability to peer farther back in time than any observatory to date, the telescope uncovered a surprising number of bright galaxies as large as the modern Milky Way within the first 500 million years, when the universe was just 3 percent of its current age.

“The bright galaxies that JWST saw would be like seeing a clustering of lights around big cities, whereas theory predicts something like the light around more rural settings like Yellowstone National Park,” Shen says. “And we don’t expect that clustering of light so early on.”

For physicists, the observations imply that there is either something fundamentally wrong with the physics underlying the models or a missing ingredient in the early universe that scientists have not accounted for. The MIT team explored the possibility of the latter, and whether the missing ingredient might be early dark energy.

Physicists have proposed that early dark energy is a sort of antigravitational force that is turned on only at very early times. This force would counteract gravity’s inward pull and accelerate the early expansion of the universe, in a way that would resolve the mismatch in measurements. Early dark energy, therefore, is considered the most likely solution to the Hubble tension.

Galaxy skeleton

The MIT team explored whether early dark energy could also be the key to explaining the unexpected population of large, bright galaxies detected by JWST. In their new study, the physicists considered how early dark energy might affect the early structure of the universe that gave rise to the first galaxies. They focused on the formation of dark matter halos — regions of space where gravity happens to be stronger, and where matter begins to accumulate.

“We believe that dark matter halos are the invisible skeleton of the universe,” Shen explains. “Dark matter structures form first, and then galaxies form within these structures. So, we expect the number of bright galaxies should be proportional to the number of big dark matter halos.”

The team developed an empirical framework for early galaxy formation, which predicts the number, luminosity, and size of galaxies that should form in the early universe, given some measures of “cosmological parameters.” Cosmological parameters are the basic ingredients, or mathematical terms, that describe the evolution of the universe.

Physicists have determined that there are at least six main cosmological parameters, one of which is the Hubble constant — a term that describes the universe’s rate of expansion. Other parameters describe density fluctuations in the primordial soup, immediately after the Big Bang, from which dark matter halos eventually form.

The MIT team reasoned that if early dark energy affects the universe’s early expansion rate, in a way that resolves the Hubble tension, then it could affect the balance of the other cosmological parameters, in a way that might increase the number of bright galaxies that appear at early times. To test their theory, they incorporated a model of early dark energy (the same one that happens to resolve the Hubble tension) into an empirical galaxy formation framework to see how the earliest dark matter structures evolve and give rise to the first galaxies.

“What we show is, the skeletal structure of the early universe is altered in a subtle way where the amplitude of fluctuations goes up, and you get bigger halos, and brighter galaxies that are in place at earlier times, more so than in our more vanilla models,” Naidu says. “It means things were more abundant, and more clustered in the early universe.”

“A priori, I would not have expected the abundance of JWST’s early bright galaxies to have anything to do with early dark energy, but their observation that EDE pushes cosmological parameters in a direction that boosts the early-galaxy abundance is interesting,” says Marc Kamionkowski, professor of theoretical physics at Johns Hopkins University, who was not involved with the study. “I think more work will need to be done to establish a link between early galaxies and EDE, but regardless of how things turn out, it’s a clever — and hopefully ultimately fruitful — thing to try.”

We demonstrated the potential of early dark energy as a unified solution to the two major issues faced by cosmology. This might be an evidence for its existence if the observational findings of JWST get further consolidated,” Vogelsberger concludes. “In the future, we can incorporate this into large cosmological simulations to see what detailed predictions we get.”

This research was supported, in part, by NASA and the National Science Foundation.



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Plant-derived secondary organic aerosols can act as mediators of plant-plant interactions

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Precision instrument bolsters efforts to find elusive dark energy


A new study published in Science reveals that plant-derived secondary organic aerosols (SOAs) can act as mediators of plant-plant interactions. This research was conducted through the cooperation of chemical ecologists, plant ecophysiologists and atmospheric physicists at the University of Eastern Finland.

It is well known that plants release volatile organic compounds (VOCs) into the atmosphere when damaged by herbivores. These VOCs play a crucial role in plant-plant interactions, whereby undamaged plants may detect warning signals from their damaged neighbours and prepare their defences. “Reactive plant VOCs undergo oxidative chemical reactions, resulting in the formation of secondary organic aerosols (SOAs). We wondered whether the ecological functions mediated by VOCs persist after they are oxidated to form SOAs,” said Dr. Hao Yu, formerly a PhD student at UEF, but now at the University of Bern.

The study showed that Scots pine seedlings, when damaged by large pine weevils, release VOCs that activate defences in nearby plants of the same species. Interestingly, the biological activity persisted after VOCs were oxidized to form SOAs. The results indicated that the elemental composition and quantity of SOAs likely determines their biological functions.

“A key novelty of the study is the finding that plants adopt subtly different defence strategies when receiving signals as VOCs or as SOAs, yet they exhibit similar degrees of resistance to herbivore feeding,” said Professor James Blande, head of the Environmental Ecology Research Group. This observation opens up the possibility that plants have sophisticated sensing systems that enable them to tailor their defences to information derived from different types of chemical cue.

“Considering the formation rate of SOAs from their precursor VOCs, their longer lifetime compared to VOCs, and the atmospheric air mass transport, we expect that the ecologically effective distance for interactions mediated by SOAs is longer than that for plant interactions mediated by VOCs,” said Professor Annele Virtanen, head of the Aerosol Physics Research Group. This could be interpreted as plants being able to detect cues representing close versus distant threats from herbivores.

The study is expected to open up a whole new complex research area to environmental ecologists and their collaborators, which could lead to new insights on the chemical cues structuring interactions between plants.



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Folded or cut, this lithium-sulfur battery keeps going

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Precision instrument bolsters efforts to find elusive dark energy


Most rechargeable batteries that power portable devices, such as toys, handheld vacuums and e-bikes, use lithium-ion technology. But these batteries can have short lifetimes and may catch fire when damaged. To address stability and safety issues, researchers reporting in ACS Energy Letters have designed a lithium-sulfur (Li-S) battery that features an improved iron sulfide cathode. One prototype remains highly stable over 300 charge-discharge cycles, and another provides power even after being folded or cut.

Sulfur has been suggested as a material for lithium-ion batteries because of its low cost and potential to hold more energy than lithium-metal oxides and other materials used in traditional ion-based versions. To make Li-S batteries stable at high temperatures, researchers have previously proposed using a carbonate-based electrolyte to separate the two electrodes (an iron sulfide cathode and a lithium metal-containing anode). However, as the sulfide in the cathode dissolves into the electrolyte, it forms an impenetrable precipitate, causing the cell to quickly lose capacity. Liping Wang and colleagues wondered if they could add a layer between the cathode and electrolyte to reduce this corrosion without reducing functionality and rechargeability.

The team coated iron sulfide cathodes in different polymers and found in initial electrochemical performance tests that polyacrylic acid (PAA) performed best, retaining the electrode’s discharge capacity after 300 charge-discharge cycles. Next, the researchers incorporated a PAA-coated iron sulfide cathode into a prototype battery design, which also included a carbonate-based electrolyte, a lithium metal foil as an ion source, and a graphite-based anode. They produced and then tested both pouch cell and coin cell battery prototypes.

After more than 100 charge-discharge cycles, Wang and colleagues observed no substantial capacity decay in the pouch cell. Additional experiments showed that the pouch cell still worked after being folded and cut in half. The coin cell retained 72% of its capacity after 300 charge-discharge cycles. They next applied the polymer coating to cathodes made from other metals, creating lithium-molybdenum and lithium-vanadium batteries. These cells also had stable capacity over 300 charge-discharge cycles. Overall, the results indicate that coated cathodes could produce not only safer Li-S batteries with long lifespans, but also efficient batteries with other metal sulfides, according to Wang’s team.

The authors acknowledge funding from the National Natural Science Foundation of China; the Natural Science Foundation of Sichuan, China; and the Beijing National Laboratory for Condensed Matter Physics.



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